I think I might be the one of the few who actually liked The High End of Low. I mean I don't really listen to half of the album tracks on it by choice, only when I'm listening to the full thing.
The High End of Low led to my my favorite song from him: Devour
but I'm actually starting to use Born Villain. It's really good for an album but if you're expecting something like golden age of grotesque then you probably won't find it as good.
My favorites on Born Villain are Pistol Whipped, Slo-Motion, Lay Down Your Goddamn Arms, Murderers are Getting Prettier Every day, and You're So Vain.
The rest are good too, but I'm not sure if I like them as much yet.